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Higher apperture lower shutter speed. Specially at dusk or dawn. (tho 2:37 pm is not near dusk). Tripod if you can use it.
And I would add doing to HDR
I like the sky and mountains
Konyan is right about the noise (grain as us film-shooters call it). Generally the lower the ISO the finer the grain. I would imagine that the CCD in your camera might have had a hard time catching full detail @ such a fast shutter speed. Next time try shooting with a smaller aperature - in this case you could have gotten away with f/11 @ 1/125 (for each stop you close down - down = bigger number - it will halve your shutterspeed. which is to say that from 5.2 to 8 you lose a 1/500 and change because it's a stop and a half, and then from 8 to 11 you lose half the shutterspeed again. I'm sure that doesn't make any sense at all).
Thank you for the detailed techical feedback - I like that kind of comment.
Oh - and the sky - it was dark, gray and gloomy everywhere else but there. . it probably lasted only a minute or two too. . . I was definitely lucky in that department.